I don’t think any tefillah is “holier” than another. They are just for different things. A tefillah is only as holy as the person davening makes it. Neilah is definitely more emotional, because it’s sort of a last chance before the gates are closed. Does that make the tefillah itself holier? I don’t think so. You can argue that mussaf, which goes through the entire avodah which was done in the Beis Hamikdash, is holier because of its contents. As I said, a tefillah is only as holy as the person davening makes it.
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